I think ND attracts a different personality. The student that is more collaborative, more team-oriented, more into school spirit, more social, eager to do community service. You know the type of kid I am talking about.
I would pick ND because the total package is better but Georgetown would be great though not nearly the experience that ND offers. And in all seriousness, the ND campus is far nicer. All this makes for a more memorable 4 years.